Thermal Properties Characterization Using Laser Flash Analysis: A Review
Abstract
Laser flash analysis (LFA) has emerged as a pivotal technique for measuring thermal diffusivity and related transport properties of materials across diverse applications. This comprehensive review examines the evolution, methodologies, and empirical applications of LFA in characterizing thermal transport phenomena. Through systematic analysis of 150 research studies spanning 2010-2024, we evaluate the effectiveness of LFA techniques across various material systems including ceramics, metals, polymers, and composites. Our empirical investigation reveals that LFA demonstrates exceptional accuracy with measurement uncertainties typically below 5% for homogeneous materials, while composite materials exhibit higher variability (8-12%). The analysis encompasses temperature-dependent measurements ranging from cryogenic conditions (-196°C) to high-temperature applications (1500°C), revealing critical insights into thermal transport mechanisms. Statistical analysis of measurement precision indicates that modern LFA systems achieve reproducibility within ±2% for standard reference materials. The review identifies emerging trends in multi-layered systems analysis, nanostructured materials characterization, and real-time monitoring applications. Comparative analysis with alternative thermal characterization methods demonstrates LFA's superior performance in rapid, non-destructive evaluation of thermal properties. This work provides a comprehensive database of thermal diffusivity values across material categories and establishes benchmark standards for future research applications.
Downloads
References
W. J. Parker, R. J. Jenkins, C. P. Butler, and G. L. Abbott, "Flash method of determining thermal diffusivity, heat capacity, and thermal conductivity," J. Appl. Phys., vol. 32, no. 9, pp. 1679-1684, 1961.
2 T. Azumi and Y. Takahashi, "Novel finite pulse-width correction in flash thermal diffusivity measurement," Rev. Sci. Instrum., vol. 52, no. 9, pp. 1411-1413, 1981.
3 L. M. Zhang, K. Liu, and M. Chen, "Thermal diffusivity measurement of ceramic matrix composites using laser flash analysis," J. Eur. Ceram. Soc., vol. 39, no. 4, pp. 1245-1253, 2019.
4 R. Kumar, S. Patel, and A. Singh, "Temperature-dependent thermal transport properties of advanced ceramics," Ceram. Int., vol. 47, no. 8, pp. 11234-11245, 2021.
5 H. Liu, J. Wang, and Z. Yang, "Comprehensive thermal diffusivity database for engineering alloys," Metall. Mater. Trans. A, vol. 51, no. 7, pp. 3456-3468, 2020.
6 D. Anderson, M. Smith, and R. Brown, "Microstructural effects on thermal transport in metallic alloys," Acta Mater., vol. 225, pp. 117589, 2022.
7 P. Wilson, T. Davis, and L. Johnson, "Thermal characterization of polymer materials using laser flash analysis," Polymer, vol. 234, pp. 124251, 2021.
8 X. Chen, Y. Li, and G. Wu, "Thermal transport in polymer composites: experimental and theoretical approaches," Compos. Sci. Technol., vol. 234, pp. 109876, 2023.
9 A. Martinez, F. Garcia, and J. Rodriguez, "Micro-flash analysis of thermal transport in nanostructured materials," Nano Lett., vol. 22, no. 12, pp. 4567-4573, 2022.
B. Thompson, K. White, and S. Green, "Interface effects in multilayer thermal transport systems," Appl. Phys. Lett., vol. 124, no. 8, pp. 081902, 2024.
11 J. R. Cowan, "Pulse method of measuring thermal diffusivity at high temperatures," J. Appl. Phys., vol. 34, no. 4, pp. 926-927, 1963.
12 L. R. Holland, "Use of black coatings to improve the accuracy of thermal diffusivity measurements," J. Appl. Phys., vol. 37, no. 11, pp. 4386-4388, 1966.
13 R. D. Cowan and J. Cowan, "Improved pulse method for measuring thermal diffusivity," Rev. Sci. Instrum., vol. 38, no. 3, pp. 394-396, 1967.
14 A. Cezairliyan, "Design and operational characteristics of a high-speed (millisecond) system for the measurement of thermophysical properties at high temperatures," J. Res. Natl. Bur. Stand., vol. 75C, no. 1, pp. 7-18, 1971.
15 R. L. Rudkin, R. J. Jenkins, and W. J. Parker, "Thermal diffusivity measurements on metals at elevated temperatures," Rev. Sci. Instrum., vol. 33, no. 1, pp. 21-24, 1962.
16 Y. S. Touloukian, R. W. Powell, C. Y. Ho, and P. G. Klemens, "Thermal conductivity of metallic elements and alloys," Thermophysical Properties of Matter, vol. 1, New York: IFI/Plenum, 1970.
17 K. D. Maglic, A. Cezairliyan, and V. E. Peletsky, "Compendium of Thermophysical Property Measurement Methods," New York: Plenum Press, 1984.
18 A. Degiovanni, "Correction of finite pulse time effects in very fast thermal diffusivity measurements," Rev. Sci. Instrum., vol. 61, no. 10, pp. 2625-2632, 1990.
19 H. Feng, "Modeling of pulse laser heating and thermal diffusivity measurement," Int. J. Heat Mass Transfer, vol. 40, no. 13, pp. 3035-3043, 1997.
20 J. E. Parrott and A. D. Stuckes, "Thermal Conductivity of Solids," London: Pion Limited, 1975.
21 M. G. Burzo, P. L. Komarov, and P. E. Raad, "Thermal transport properties of gold-covered thin-film silicon dioxide," IEEE Trans. Compon. Packag. Technol., vol. 26, no. 1, pp. 80-88, 2003.
22 S. M. Lee and D. G. Cahill, "Heat transport in thin dielectric films," J. Appl. Phys., vol. 81, no. 6, pp. 2590-2595, 1997.